Chirality Assignment of Micelle-Suspended Single-Walled Carbon Nanotubes Using Coherent Phonon Oscillations

نویسندگان

  • Yong-Sik Lim
  • Ji-Hee Kim
  • Erik H. Hároz
  • Jonah Shaver
  • Junichiro Kono
  • Stephen K. Doorn
  • Robert H. Hauge
  • Richard E. Smalley
چکیده

We report on a new high-resolution optical spectroscopy, coherent phonon measurement, for determining the chiral index of carbon nanotubes. Using femtosecond pump-probe spectroscopy, we demonstrate the real-time observation of lattice vibrations in individualized single-walled carbon nanotubes in an aqueous surfactant solution. Almost all available radial breathing modes in the Fourier transform spectrum from coherent phonon oscillations are well-resolved with less ambiguity in comparison to continuous-wave resonant Raman scattering.

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تاریخ انتشار 2007